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Visible light induced photoacid generation within plasticized PVC membranes for copper (II) ion extraction
Journal article   Peer reviewed

Visible light induced photoacid generation within plasticized PVC membranes for copper (II) ion extraction

Xiaojiang Xie, Gunter Mistlberger and Eric Bakker
Sensors and Actuators B: Chemical, Vol.204, pp.807-810
2014
url
https://doi.org/10.1016/j.snb.2014.08.041View
Published Version

Abstract

Analytical Chemistry Materials Engineering Optical Physics photoacid generator copper camphorquinone PVC
We present here an approach for light induced generation of lipophilic cation-exchangers in plasticized PVC membranes. Using camphorquinone as photosensitizer, a lipophilic cationic photoacid generator can produce protons under visible light illumination and endow the polymeric membrane with ion-exchanging property. After light illumination, the membrane containing a Cu2+ ionophore, is able to extract Cu2+ ions from the contacting aqueous solution. The acid generation upon light irradiation is relatively fast (ca. 100 s). The Cu2+ extraction process was imaged with fluorescence microscopy using Calcein, a fluorescence indicator whose fluorescence is quenched by Cu2+. Such a technique may form a new platform for light triggered ion concentration perturbation.

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