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Towards Ion-Selective Membranes with Electrogenerated Chemiluminescence Detection: Visualizing Selective Ru(bpy)32+ Transport Across a Plasticized Poly(vinyl chloride) Membrane
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Towards Ion-Selective Membranes with Electrogenerated Chemiluminescence Detection: Visualizing Selective Ru(bpy)32+ Transport Across a Plasticized Poly(vinyl chloride) Membrane

G A Crespo, G Mistlberger and Eric Bakker
Electroanalysis, Vol.24(1), pp.61-68
2012
url
https://doi.org/10.1002/elan.201100434View
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Abstract

ion-selective membranes electrogenerated chemiluminescence (ECL) ion-selective transport chemical imaging
We report here on an attractive concept to integrate electrochemically triggered ion-selective transport across an ion-selective plasticized PVC membrane and electrogenerated chemiluminescence (ECL) as a detection technique. This will eventually form the basis for an alternate transduction mechanism for electrochemical ion sensors. To this end, the selective extraction of the ECL reagent Ru(bpy)32+ is demonstrated by an o-NPOE plasticized PVC membrane doped with lipophilic cation-exchanger. Chemical imaging of Ru(bpy)32+ electrotransported across the PVC membrane demonstrates the feasibility of this concept as a future trend for two dimensional ion sensing.

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Web Of Science research areas
Chemistry, Analytical
Electrochemistry
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