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Concanavalin A electrochemical sensor based on the surface blocking principle at an ion-selective polymeric membrane
Journal article   Peer reviewed

Concanavalin A electrochemical sensor based on the surface blocking principle at an ion-selective polymeric membrane

M Pawlak, G Mistlberger and Eric Bakker
Microchimica Acta, Vol.182(1-2), pp.129-137
2015
url
https://doi.org/10.1007/s00604-014-1309-3View
Published Version

Abstract

Analytical Chemistry Other Chemical Sciences biosensor chronopotentiometry click chemistry concanavalin A ion selective electrodes
We report on a new electrochemical sensor for Concanavalin A. It is based on blocking the surface of plasticized PVC membranes that were covalently modified with D-mannose using click chemistry. The interaction of D-mannose with Concanavalin A on the surface perturbs the flux of a marker ion for which the ion-selective membrane is responsive, and this results in a change in the electrochemical signal. The sensor was characterized using a variety of electrochemical protocols, and results were confirmed by quartz crystal microbalance experiments. The lowest limit of detection (10 μg mL-1) was obtained using a membrane containing a cation exchanger and tetrabutylammonium ion as the marker ion. [Figure not available: see fulltext.] © 2014 Springer-Verlag Wien.

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