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Asymmetric Synthesis of Indole Homo-Michael Adducts via Dynamic Kinetic Friedel-Crafts Alkylation with Cyclopropanes
Journal article   Peer reviewed

Asymmetric Synthesis of Indole Homo-Michael Adducts via Dynamic Kinetic Friedel-Crafts Alkylation with Cyclopropanes

Steven M. Wales, Morgan M. Walker and Jeffrey S. Johnson
Organic Letters, Vol.15(10), pp.2558-2561
2013
PMID: 23654283
url
https://doi.org/10.1021/ol4010646View
Published Version

Abstract

alcohols hydrocarbons indoles Lewis acids post-translational modification
An enantioconvergent Friedel-Crafts alkylation of indoles with donor-acceptor cyclopropanes is described. The reaction is catalyzed by pybox center dot Mgl(2) and proceeds via a type I dynamic kinetic asymmetric transformation (DyKAT).

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Chemistry, Organic

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